The Little Mix singer has also unfollowed Zayn on the band’s Twitter page, following the news earlier this week that he had called time on their relationship, two years after they announced that they were engaged.
During their relationship, Perrie’s Instagram page was one of the few places that fans could get a look at the couple, who were rarely photographed in public together.
Earlier this year, it was on Perrie’s Instagram that Zayn first showed off his newly-dyed green hair, while they also shared snaps from their holiday together, shortly after he announced that he had quit One Direction.
However, she’s now removed all pictures of him from her social media page, severing ties with him even further.
Perrie, meanwhile, recently said she was “doing good”, when quizzed by an American reporters about how she was coping with the break-up.
While promoting their latest single, ‘Black Magic’, in the US, Perrie’s bandmates were seen trying to cheer her up, with Leigh-Anne Pinnock even putting on a show for paparazzi photographers, so they weren’t able to get a glum-looking photo of her friend.